Strangers in the Night - S6-E12
Character mistake: The whole idea of the serenading scene was Larry was supposed to hide and sing for Jack while Jack would be shown in the yard alone and pretend to be the one singing, but the yard was brightly lit and Larry was right behind Jack and both were very shown with nothing to hide Larry.
Answer: I believe you are referring to the artwork of Alphonse Mucha. On the wall next to the front door was "Feather" (which is one half of "Primrose and Feather"). Above the telephone in early episodes was "Zodiac". Also seen through The Apartment was "Spring" and "Autumn".